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Stabilization of U 5f2 configuration in UTe2 through U 6d dimers in the presence of Te2 chains

Denise S. Christovam1, Martin Sundermann1,2, Andrea Marino1, Daisuke Takegami1,*, Johannes Falke1, Paulius Dolmantas1, Manuel Harder3,4, Hlynur Gretarsson2,5, Bernhard Keimer5 et al.

Andrei Gloskovskii2, Maurits W. Haverkort6, Ilya Elfimov7, Gertrud Zwicknagl1,8, Alexander V. Andreev9, Ladislav Havela10, Mitchell M. Bordelon11, Eric D. Bauer11, Priscila F. S. Rosa11, Andrea Severing1,12, and Liu Hao Tjeng1

  • *Present address: Department of Applied Physics, Waseda University, Shinjuku, Tokyo 169-8555, Japan.
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Phys. Rev. Research 6, 033299 – Published 16 September, 2024

DOI: https://doi.org/10.1103/PhysRevResearch.6.033299

Abstract

We investigate the topological superconductor candidate UTe2 using high-resolution valence-band resonant inelastic x-ray scattering at the U M4,5 edges. We observe atomiclike low-energy excitations that support the correlated nature of this unconventional superconductor. These excitations originate from the U 5f2 configuration, which is unexpected since the short Te2-Te2 distances exclude Te2 being 2−. By utilizing the photoionization cross-section dependence of the photoemission spectra in combination with band structure calculations, we infer that the stabilization of the U 5f2 configuration is due to the U 6d bonding states in the U dimers acting as a charge reservoir. Our results emphasize that the description of the physical properties should commence with a 5f2 ansatz.

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Phys. Rev. Research 6, 033299– Published 16 September, 2024
  • Received 29 January 2024
  • Accepted 23 August 2024
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